Authors
Anika Kinkhabwala, Zongfu Yu, Shanhui Fan, Yuri Avlasevich, Klaus Müllen, William E Moerner
Publication date
2009/11
Journal
Nature photonics
Volume
3
Issue
11
Pages
654-657
Publisher
Nature Publishing Group UK
Description
Owing to the size mismatch between light and nanoscale objects such as single molecules, it is important to be able to control light–molecule interactions,,,. Plasmonic nanoantennas create highly enhanced local fields when pumped resonantly, leading to increased Raman scattering, but whether fluorescence enhancement occurs depends upon a variety of factors. Although sharp metal tips and colloids, can enhance fluorescence, the highly enhanced optical fields of lithographically fabricated bowtie nanoantennas provide a structure that is more controllable and amenable to integration. Using gold bowties, we observe enhancements of a single molecule's fluorescence up to a factor of 1,340, ten times higher than reported previously,,,,,,,,,,,,,,. Electromagnetic simulations reveal that this is a result of greatly enhanced absorption and an increased radiative emission rate, leading to enhancement of the intrinsic …
Total citations
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Scholar articles
A Kinkhabwala, Z Yu, S Fan, Y Avlasevich, K Müllen… - Nature photonics, 2009